Personally I had more trouble with Game of Life and 2 of Kaguya's last spells than either of those, but you're close. At the rate you're going it shouldn't take too long.
Also I had the horrible idea of trying to get a 'perfect' IN score.dat, involving
4860 different 1ccs (all difficulties with all teams/solos)
Easy and normal are trivial, I already did extra, most of hard won't be too bad, and I just got the last team lunatic 1cc today (Scarlet team)
Said run had the WORST Wriggle battle ever, the BEST Mystia, the BEST Keine, a predictably bad Reimu because I have almost 0 practice with her, an ok Reisen, a HORRENDOUS Eirin (3 bombs, a life, and 2 more bombs? that's what I used on Reisen...), and a fantastic Kaguya, but not as good as my Magic team run of her.
If I recall correctly, that unlocks one the most god-awful spells in the history of Touhou...
Good luck! 
Fantasy Heaven...Be prepared for a several hour grind to figure out where to go when, wait for Reimu to move the right direction and not screw up. Although when I captured it I was set for another 2-3 seconds, so...